Enhancing perovskite-silicon tandem solar cells through numerical optical and electric optimizations for light...

We integrated optical and electrical numerical simulations to precisely investigate the effectiveness of using a pyramidal perovskite (Cs_0.18FA_0.82Pb(I,Br)₃) nanostructured film as an example in perovskite-silicon tandem solar cells to reduce reflective losses and balance the current densities. Through our calculations, the PCE of tandem solar cells can be improved from 29.2% (the planar structures without texturing) to 36.1% in the best-performing textured tandem devices under the consistently calculated absorbed and EQE spectrum, where the predicted open-circuit voltage could reach over 2 V. These findings offer valuable theoretical insights for the advancement and optimization of perovskite-silicon tandem solar cells.