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Engineered Nanoporous Frameworks for Adsorption Cooling Applications.

Jian Shen^1,2, Abhishek Kumar¹, Mohammad Wahiduzzaman³

¹Energy and Environment Directorate, Pacific Northwest National Laboratory, Richland, Washington 99352, United States.

Chemical Reviews

|April 29, 2024

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Engineered nanoporous frameworks (ENFs) offer a promising sustainable solution for adsorption cooling, addressing rising energy demands. Research highlights ENF-refrigerant interactions and selection factors for efficient, eco-friendly cooling technologies.

Area of Science:

Materials Science
Chemical Engineering
Thermodynamics

Background:

Rising global energy demand for space cooling driven by global warming and population growth necessitates sustainable alternatives.
Traditional vapor-compression cooling is energy-intensive, prompting a search for eco-friendly technologies utilizing waste or sustainable energy.
Adsorption cooling presents a viable alternative, but requires advanced materials for efficient refrigerant sorption.

Purpose of the Study:

To review refrigerants and sorbents for adsorption cooling.
To focus on engineered nanoporous frameworks (ENFs) and their refrigerant pairs for enhanced adsorption cooling.
To analyze factors influencing ENF-refrigerant selection and interaction mechanisms.

Main Methods:

Review of existing literature on refrigerants, sorbents, and adsorption cooling cycles.

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Last Updated: Jun 27, 2025

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Analysis of studies employing engineered nanoporous frameworks (ENFs) with various refrigerants.

Discussion of characterization techniques and computational modeling for understanding sorbent-refrigerant interactions.

Examination of ENF properties such as pore structure, chemistry, and morphology.

Main Results:

Identified limitations of traditional sorbents, emphasizing the need for advanced materials.
Detailed the effects of ENF properties (pore size, chemistry, morphology) on refrigerant selection and performance.
Provided insights into sorbent-refrigerant interactions and pore-filling mechanisms.
Highlighted the potential of ENFs in improving adsorption cooling efficiency.

Conclusions:

Engineered nanoporous frameworks (ENFs) show significant promise for advanced adsorption cooling applications.
Optimizing ENF-refrigerant pairs through understanding material properties and interactions is crucial for efficient, sustainable cooling.
Further research into challenges and opportunities will drive the future development of ENF-based adsorption cooling technology.