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Transition between Heavy-Fermion-Strange-Metal and Quantum Spin Liquid in a 4d-Electron Trimer Lattice
Hengdi Zhao1, Yu Zhang1, Pedro Schlottmann2
1Department of Physics, University of Colorado at Boulder, Boulder, Colorado 80309, USA.
Abstract:
We present experimental evidence that a heavy Fermi surface consisting of itinerant, charge-neutral spinons underpins both heavy-fermion-strange-metal (without f electrons) and quantum-spin-liquid states in the 4d-electron trimer lattice, Ba_{4}Nb_{1-x}Ru_{3+x}O_{12}(|x|<0.20). These two exotic states both exhibit an extraordinarily large entropy, a linear heat capacity extending into the milli-Kelvin regime, a linear thermal conductivity at low temperatures, and separation of charges and spins. Furthermore, the insulating spin liquid is a much better thermal conductor than the heavy-fermion-strange-metal that separately is observed to strongly violate the Wiedemann-Franz law. We propose that at the heart of this 4d system is a universal, heavy spinon Fermi surface that provides a unified framework for explaining the exotic phenomena observed throughout the entire series. The control of such exotic ground states provided by variable Nb concentration offers a new paradigm for studies of correlated quantum matter.
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