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Realization of Long-Life Proton Battery by Layer Intercalatable Electrolyte.

Peilin Liang1,2,3, Shuanlong Di4, Yuxin Zhu4

  • 1School of Metallurgy, Northeastern University, Shenyang, 110819, P. R. China.

Angewandte Chemie (International Ed. in English)
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Summary

Researchers developed a novel layer intercalatable electrolyte (LIE) for proton batteries, overcoming water corrosion issues. This innovation enhances battery safety and performance, especially at low temperatures.

Keywords:
intercalatable electrolytelow water activitylow-temperature cyclingproton batterysolvation structure

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Area of Science:

  • Electrochemistry
  • Materials Science
  • Energy Storage

Background:

  • Proton batteries offer safe, low-temperature grid-scale energy storage.
  • Electrolyte design is hindered by free water corrosion, limiting development.

Purpose of the Study:

  • To develop a novel electrolyte for proton batteries that mitigates corrosion and improves performance.
  • To introduce a new working mechanism for proton reactions in aqueous batteries.

Main Methods:

  • Formulation of a layer intercalatable electrolyte (LIE) by incorporating trimethyl phosphate (TMP) into acidic electrolytes.
  • Investigation of the co-intercalation of solvent molecules into anode material interlayers.
  • Electrochemical testing of half-cells and full-cell batteries.

Main Results:

  • The LIE enabled co-intercalation, establishing a new proton reaction mechanism.
  • Electrode corrosion was significantly reduced, expanding the electrochemical stability window.
  • Half-cells demonstrated 91.0% capacity retention after 5000 cycles at 5 A/g.
  • Full batteries maintained 74.9% capacity for 2 months at -20°C.

Conclusions:

  • The developed LIE offers a promising solution for overcoming corrosion in aqueous batteries.
  • This work opens new avenues for designing advanced electrolytes for proton batteries.
  • The enhanced low-temperature performance and cycling stability are critical for grid-scale applications.