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Engineering valence-mismatched Ti4+ into Fe-based metal-organic-frameworks for enhanced photocatalytic CO2 reduction
Rui Li1, Xiang Xue1, Minqi Wu1
1College of Environment, Zhejiang University of Technology, Hangzhou 310014, China.
Chemical Communications (Cambridge, England)
|July 17, 2024
Abstract:
A series of low-dose high-valence Ti4+ doped MIL-53-NH2(Fe) photocatalysts were synthesized for visible-light-driven CO2 reduction. The highest CO2-to-CO conversion rate of Ti4+ doped MIL-53-NH2(Fe) was 7.24 mmol g-1 h-1 and the highest CO selectivity was 94% in acetonitrile solvent using [Ru(bpy)3]2+ and triethanolamine.
