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Formation of Complex Ions03:45

Formation of Complex Ions

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A type of Lewis acid-base chemistry involves the formation of a complex ion (or a coordination complex) comprising a central atom, typically a transition metal cation, surrounded by ions or molecules called ligands. These ligands can be neutral molecules like H2O or NH3, or ions such as CN− or OH−. Often, the ligands act as Lewis bases, donating a pair of electrons to the central atom. These types of Lewis acid-base reactions are examples of a broad subdiscipline called coordination...
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Solid-state Graft Copolymer Electrolytes for Lithium Battery Applications
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Rationally Designed Li-Ag Alloy with In-Situ-Formed Solid Electrolyte Interphase for All-Solid-State Lithium

Ye-Eun Park1, Myung-Keun Oh2, Hui-Tae Sim2

  • 1Department of Battery Engineering, Hanyang University, Seoul 04763, Republic of Korea.

ACS Applied Materials & Interfaces
|July 22, 2024
PubMed
Summary
This summary is machine-generated.

Researchers developed a novel lithium-silver (Li-Ag) alloy anode for all-solid-state lithium batteries (ASSLBs). This Li-Ag anode with a protective interphase layer effectively suppresses lithium dendrites, enhancing battery safety and performance.

Keywords:
all-solid-state lithium batterieselectrodepositionlithium dendritelithium−silver alloysolid electrolyte interphase

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • All-solid-state lithium batteries (ASSLBs) using sulfide electrolytes offer high energy density and safety.
  • Challenges include lithium dendrite growth and side reactions at the lithium metal anode-sulfide electrolyte interface.
  • These issues degrade ASSLB performance and pose safety risks.

Purpose of the Study:

  • To develop a stable lithium metal anode for ASSLBs.
  • To mitigate performance degradation caused by lithium dendrites and interfacial side reactions.
  • To improve the overall safety and cycling stability of ASSLBs.

Main Methods:

  • Preparation of a silver-based lithium (Li-Ag) alloy anode via electrodeposition.
  • Characterization of the electrochemically formed solid electrolyte interphase (SEI) layer on the Li-Ag alloy.
  • Assembly and testing of symmetric cells and full ASSLB cells using the Li-Ag anode.

Main Results:

  • The SEI layer on the Li-Ag alloy, composed of LiF, Li2O, and Li3N, exhibited high mechanical strength and ionic conductivity.
  • The Li-Ag alloy anode successfully suppressed lithium dendrite formation and cell short-circuiting.
  • Symmetric cells demonstrated a critical current density of 1.6 mA cm-2 and stable cycling over 2000 hours.
  • A full ASSLB with the Li-Ag anode delivered a high discharge capacity of 185 mAh g-1 with good cycling stability and rate capability.

Conclusions:

  • The developed Li-Ag alloy anode with a robust SEI layer is a promising solution for stable ASSLBs.
  • This anode design effectively addresses the critical challenges of lithium dendrite growth and interfacial instability.
  • The findings pave the way for safer and higher-performance all-solid-state lithium batteries.