CO₂-Accelerated Carbonation Modification for Recycled Coarse Aggregate with Various Original Concrete Strengths and...

The increasing demand for concrete reduces natural resources, such as sand and gravel, and also leads to a sharp increase in the amount of waste concrete produced. Due to the fact that the physical and mechanical properties of waste concrete made of recycled aggregates (RAs) differ greatly, it is difficult to use directly as a raw material for reinforced concrete (RC) components, which greatly restricts the popularization and application of RAs in actual projects. Utilizing the alkali aggregate properties of RAs to capture CO₂ from industrial waste gases is an innovative way of enhancing their properties and promoting their application in real projects. However, the extent of the influence of original concrete strength (OCS) and coarse aggregate size (CAS) on the accelerated carbonation modification of RA is not clear, and a quantitative description is still required. For this purpose, accelerated carbonation tests on recycled coarse aggregate (RCA) samples under completely dry condition were carried out, and the variation laws for the physical property indicators of RCA samples before and after accelerated carbonation versus the OCS and CAS were revealed. Moreover, the influence degrees of the two factors, OCS and CAS, on the property enhancement of RCAs after accelerated carbonation were clarified, and the results of OCS and CAS corresponding to the best accelerated carbonation effects of RCAs were determined. By analyzing the micromorphology of RCA before and after accelerated carbonation, the reasons for property enhancement of RCAs with various OCSs and CASs under the best carbonation modifications were clarified. The findings will contribute to the development of basic theoretical research on accelerated carbonation modification of RA and have important scientific value.