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Room-Temperature Self-Healing and Recyclable Self-Crosslinked Isosorbide-Based Adhesive Bioelastomer.

Qing Ouyang1, Ming-Xuan Du1, Yao-Nan Xiao1

  • 1CAS Key Laboratory of Engineering Plastics, Beijing National Laboratory for Molecular Sciences, Institute of Chemistry, the Chinese Academy of Sciences, Beijing, 100190, China.

Macromolecular Rapid Communications
|August 16, 2024
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Summary

New bioelastomers derived from isosorbide (PICBAs) offer excellent self-healing and adhesive properties. These renewable materials show great potential as eco-friendly pressure-sensitive adhesives (PSAs).

Keywords:
adhesivebio‐basedelastomerrecyclableself‐healing

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Area of Science:

  • Materials Science
  • Polymer Chemistry
  • Green Chemistry

Background:

  • Growing environmental concerns necessitate the development of sustainable, renewable materials.
  • Bio-based polymers are gaining traction as alternatives to petroleum-based plastics.
  • Isosorbide is a promising renewable monomer derived from plant starch.

Purpose of the Study:

  • To synthesize and characterize novel isosorbide-based bioelastomers.
  • To evaluate the mechanical, self-healing, and adhesive properties of these bioelastomers.
  • To explore their potential application as environmentally friendly pressure-sensitive adhesives (PSAs).

Main Methods:

  • Facile and economical two-step melt polycondensation was employed for synthesis.
  • Poly(isosorbide carbonate-co-butanediol aliphatic esters)s (PICBAs) were synthesized.
  • Mechanical testing, self-healing evaluation, and adhesion tests were conducted.

Main Results:

  • PICBAs demonstrated excellent tensile strength and remarkable self-healing capabilities, with over 95% recovery after 48 hours at room temperature.
  • The synthesized bioelastomers exhibited strong adhesive performance on various substrates, outperforming commercial double-sided tape.
  • A slight self-crosslinking reaction of isosorbide contributed to the observed properties.

Conclusions:

  • Isosorbide-based bioelastomers (PICBAs) are synthesized efficiently via melt polycondensation.
  • PICBAs possess superior mechanical and self-healing properties, along with excellent adhesion.
  • These bioelastomers show significant promise for application as sustainable, high-performance pressure-sensitive adhesives (PSAs).