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Double-Sided Pressure-Sensitive Adhesive Materials under Human-Centric Extreme Environments.

Jisoo Jeon1, Jinyoung Kim1, Sehyun Park1

  • 1School of Materials Science and Engineering, Georgia Institute of Technology, Atlanta, Georgia 30332, United States.

ACS Applied Materials & Interfaces
|September 2, 2024
PubMed
Summary

Flexible pressure-sensitive adhesives (PSAs) for wearable sensors maintain adhesion under extreme conditions. Temperature, moisture, and stress impact PSA performance, influencing device reliability for health monitoring.

Keywords:
human-centric extreme environmentlap shear testlong-term adhesion stabilitypressure-sensitive adhesivewearable sensors

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Area of Science:

  • Materials Science
  • Biomedical Engineering
  • Adhesion Science

Background:

  • Flexible pressure-sensitive adhesives (PSAs) are vital for wearable sensor devices, especially in health monitoring applications.
  • Sustainable mounting of these devices is critical under diverse and challenging environmental conditions.

Purpose of the Study:

  • To investigate the adhesive, mechanical, and optical properties of medical-grade double-sided PSAs.
  • To simulate and evaluate PSA performance in extreme human-centric environments, including temperature variations, moisture, and mechanical stress.

Main Methods:

  • Tested medical-grade double-sided PSAs under diverse temperature conditions (low and high).
  • Exposed PSAs to water immersion (salty, weakly acidic) and high humidity for up to 28 days.
  • Applied cyclical shear loads and analyzed failure modes (adhesive vs. cohesive) and property changes.

Main Results:

  • High temperatures increased shear adhesion strength; low temperatures reduced it by hardening the adhesive.
  • Water immersion and humidity decreased adhesion due to interference with interfacial interactions.
  • Extreme mechanical stresses and cyclical loading led to adhesive or cohesive failure, influenced by polar solvents.

Conclusions:

  • PSA performance is directly linked to morphological changes, surface roughness, swelling, and contact area alterations.
  • Findings provide design guidelines for robust wearable human health monitoring sensors for long-term applications.
  • Understanding these relationships is key to developing reliable wearable devices and electrodes.