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Related Concept Videos

Interference and Diffraction02:18

Interference and Diffraction

Interference is a characteristic phenomenon exhibited by waves. When two electromagnetic waves interact with their peaks and troughs coinciding, a resulting wave with enhanced amplitude is produced. This is known as constructive interference. In this case, the two waves interacting are in phase with each other.

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Interference between multipolar two-photon transitions in quantum emitters near plasmonic nanostructures.

S Smeets1, B Maes2, G Rosolen2

  • 1Micro- and Nanophotonic Materials Group, Research Institute for Materials Science and Engineering, University of Mons, 20 Place du Parc, 7000, Mons, Belgium. Steve.Smeets@umons.ac.be.

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|September 27, 2024
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Summary

We developed a new framework to model interference in two-photon spontaneous emission (TPSE) near nanostructures. This approach reveals how multipolar pathways can enhance or suppress TPSE, offering new design possibilities.

Keywords:
Dipole approximation breakdownFrameworkInterferencePlasmonic nanostructurePurcell factorTwo-photon spontaneous emission

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Area of Science:

  • Quantum optics
  • Plasmonics
  • Nanophotonics

Background:

  • Spontaneous emission near plasmonic nanostructures involves complex multipolar pathways beyond simple dipole emission.
  • Two-photon spontaneous emission (TPSE) exhibits higher-order multipolar emission channels that can interfere.
  • Understanding these interference effects is crucial for controlling light-matter interactions at the nanoscale.

Purpose of the Study:

  • To develop a novel computational framework for analyzing interference effects in TPSE near arbitrary nanostructures.
  • To investigate the breakdown of dipolar selection rules in TPSE due to enhanced multipolar transitions.
  • To provide a tool for designing quantum emitters and nanostructures for tailored TPSE.

Main Methods:

  • Developed a framework based on calculating Purcell factors using conventional electromagnetic simulations.
  • Avoided complex analytical calculations by leveraging established simulation techniques.
  • Applied the framework to a hydrogen-like emitter near a graphene nanotriangle.

Main Results:

  • Demonstrated a breakdown of the dipolar selection rule in TPSE near a graphene nanotriangle.
  • Observed significant enhancement of two-electric dipole (2ED) and two-electric quadrupole (2EQ) transitions.
  • Quantified the impact of interference between multipolar transitions, showing an increase in the total emission rate.

Conclusions:

  • The developed framework accurately computes interference effects in TPSE near nanostructures.
  • Multipolar transitions and their interference play a significant role in TPSE, challenging dipolar selection rules.
  • Exploiting these interference effects offers a new degree of freedom for enhancing or suppressing specific TPSE pathways.