Robust second-order topological insulator in 2D van der Waals magnet CrI3
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Updated: Jun 11, 2025

Fabricating van der Waals Heterostructures with Precise Rotational Alignment
Published on: July 5, 2019
Xiaorong Zou1, Yingxi Bai1, Ying Dai1
1School of Physics, State Key Laboratory of Crystal Materials, Shandong University, Jinan 250100, China. daiy60@sdu.edu.cn.
Abstract:
CrI3 offers an intriguing platform for exploring fundamental physics and the innovative design of spintronics devices in two-dimensional (2D) magnets, and moreover has been instrumental in the study of topological physics. However, the 2D CrI3 monolayer and bilayers have long been thought to be topologically trivial. Here we uncover a hidden facet of the band topology of 2D CrI3 by showing that both the CrI3 monolayer and bilayers are second-order topological insulators (SOTIs) with a nonzero second Stiefel-Whitney number w2 = 1. Furthermore, the topologically nontrivial nature can be explicitly confirmed via the emergence of floating edge states and in-gap corner states. Remarkably, in contrast to most known magnetic topological states, we put forward that the SOTIs in 2D CrI3 monolayer and bilayers are highly robust against magnetic transitions, which remain intact under both ferromagnetic and antiferromagnetic configurations. These interesting predictions not only provide a comprehensive understanding of the band topology of 2D CrI3 but also offer a favorable platform to realize magnetic SOTIs for spintronics applications.
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