Anomalous Metamagnetism in the Low Carrier Density Kondo Lattice YbRh₃Si₇

We report complex metamagnetic transitions in single crystals of the new low carrier Kondo antiferromagnet ${\text{YbRh}}_3{\text{Si}}_7$ . Electrical transport, magnetization, and specific heat measurements reveal antiferromagnetic order at $T_{\text{N}}=7.5K$ . Neutron diffraction measurements show that the magnetic ground state of ${\text{YbRh}}_3{\text{Si}}_7$ is a collinear antiferromagnet, where the moments are aligned in the ab plane. With such an ordered state, no metamagnetic transitions are expected when a magnetic field is applied along the $c$ axis. It is therefore surprising that high-field magnetization, torque, and resistivity measurements with $H\Vert c$ reveal two metamagnetic transitions at ${\mathrm{micro}}_0{H}_1=6.7\text{T}$ and ${\mathrm{micro}}_0{H}_2=21\text{T}$ . When the field is tilted away from the $c$ axis, towards the ab plane, both metamagnetic transitions are shifted to higher fields. The first metamagnetic transition leads to an abrupt increase in the electrical resistivity, while the second transition is accompanied by a dramatic reduction in the electrical resistivity. Thus, the magnetic and electronic degrees of freedom in ${\text{YbRh}}_3{\text{Si}}_7$ are strongly coupled. We discuss the origin of the anomalous metamagnetism and conclude that it is related to competition between crystal electric-field anisotropy and anisotropic exchange interactions.