Recent advances in regulation methods for selective separation and precise control of two-dimensional (2D) lamellar...

Selective separation and precise control of the structure and surface characterization for two-dimensional (2D) membranes is the key technology that needs to be revealed for further development of the material in practical application. Current researches focus on the cross-linking and modification of single nanosheet to improve and manipulate the performance of 2D lamellar membranes. In this paper, the selectivity principles such as size exclusion, charge properties, and surface chemical affinity in the separation process of 2D membranes were comprehensively and systematically reviewed, as well as the preparation of hybrid membranes combining the advantages of various raw materials. We also analyzed the practical application of the separation principles in relevant researches and discussed the development directions of 2D membranes. These inductions have certain summary and guiding significance for the selective regulation and goal-oriented design of 2D membranes.