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Updated: Jun 7, 2025

Measurement of Coherence Decay in GaMnAs Using Femtosecond Four-wave Mixing
Published on: December 3, 2013
Suppressed Nonreciprocal Second-Harmonic Generation of Antiferromagnet MnPSe3 in the MnPSe3/Graphene Heterostructure
Ziyun Wang1,2, Yuqiang Liu1,3, De Hou1
1High Magnetic Field Laboratory, HFIPS, Chinese Academy of Sciences, Hefei 230031, P. R. China.
Abstract:
Interfacial coupling is one of the keys to manipulating magnetic/nonmagnetic two-dimensional (2D) heterostructures for novel functionalities. The MnPSe3/graphene heterostructure is a prospective platform for quantum information and metrology. However, how graphene affects MnPSe3 through interfacial coupling is still poorly understood. Herein, second-harmonic generation (SHG) of antiferromagnet MnPSe3 in the MnPSe3/graphene heterostructure is revealed. Surprisingly, it was found that below TN, nonreciprocal or c-type SHG of MnPSe3 disappeared when interfacing with the graphene, suggesting the existence of interfacial couplings and/or interactions. Most interestingly, different from the short-range interfacial proximity interaction, this interfacial interaction could be contactless and long-range and varied from 2D metallic/semiconducting to insulating underlayers. Interfacial magnon-plasmon coupling probably played an important role in suppressing the c-type SHG signals of MnPSe3 in the MnPSe3/graphene heterostructure. This study will improve our understanding of the manipulation of nonlinear optical properties in 2D heterostructures.
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