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Surface Plasmons in Two-Dimensional MXenes.

Calvin Raab^1,2, Janek Rieger¹, Atreyie Ghosh¹

¹James Franck Institute, University of Chicago, Chicago, Illinois 60637, United States.

The Journal of Physical Chemistry Letters

|November 14, 2024

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Imaging and simulation of surface plasmon polaritons on layered 2D MXenes.

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MXenes, a novel class of 2D materials, show great potential for plasmonics due to their tunable properties. This study clarifies plasmon behavior in MXenes and explores new research directions for advanced photonic applications.

Area of Science:

Materials Science
Condensed Matter Physics
Nanotechnology

Background:

MXenes are 2D transition metal carbides/nitrides with tunable optoelectronic properties.
Their metallic nature and conductivity make them suitable for 2D plasmonics.
Applications include catalysis, SERS, and electromagnetic shielding, but synthetic complexity poses challenges.

Purpose of the Study:

To clarify plasmon physics in MXenes, particularly addressing disagreements in the prototypical Ti3C2Tx.
To explore the potential of hyperbolic plasmons in MXenes.
To propose new research avenues for MXene photonics.

Main Methods:

Applying fundamental models and theories of plasmon physics to MXenes.
Analyzing the properties of MXene chemical structures for plasmonic tuning.

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Reviewing existing literature and experimental data on MXene plasmon resonances.

Main Results:

Provided a clearer understanding of plasmon energy and resonance assignments in MXenes.
Identified the potential for hyperbolic plasmons in various MXene compositions.
Highlighted the tunability of MXene properties for specific plasmonic applications.

Conclusions:

MXenes offer a versatile platform for advanced plasmonic devices.
Further research into hyperbolic plasmons could unlock novel photonic functionalities.
Addressing synthetic challenges is key to realizing MXene plasmonics in applications.