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Adaptive Opto-Thermal-Hydrodynamic Manipulation and Polymerization (AOTHMAP) for 4D Colloidal Patterning
Yang Shi1, Lianrou Liu1, Jingping Huang1
1Guangdong Provincial Key Laboratory of Nanophotonic Manipulation, Institute of Nanophotonics, College of Physics & Optoelectronic Engineering, Jinan University, Guangzhou, 511443, P. R. China.
Advanced Materials (Deerfield Beach, Fla.)
|November 15, 2024
Summary
A novel 4D colloidal patterning method (AOTHMAP) uses a single laser to precisely assemble microstructures. This adaptive opto-thermal-hydrodynamic technique enables complex 1D, 2D, and 3D designs with dynamic shape changes for advanced applications.
Area of Science:
- Colloidal science
- Materials science
- Microfabrication
Background:
- Precision colloidal patterning is crucial for micro/nanostructures in manufacturing, optoelectronics, and biofabrication.
- Existing methods often lack versatility or require complex setups.
Purpose of the Study:
- To report a direct 4D patterning method with single-particle resolution.
- To demonstrate a versatile and efficient strategy for constructing customizable colloidal microstructures.
Main Methods:
- Developed adaptive opto-thermal-hydrodynamic manipulation and polymerization (AOTHMAP) using a single laser beam.
- Utilized light-induced hydrodynamic force, optical force, and photothermal polymerization for particle manipulation.
- Incorporated pH-responsive hydrogel adhesives for dynamic 4D patterning capabilities.
Main Results:
- Achieved precise 1D, 2D, and 3D patterning of various colloidal particles.
- Demonstrated the construction of complex microstructures with customizable shapes.
- Enabled dynamic 4D patterning through shrinkage, restructuring, and cloaking.
- Successfully patterned functional bio-structures, including bio-micromotors.
Conclusions:
- AOTHMAP provides a simple, efficient, and versatile strategy for colloidal patterning.
- The method holds significant promise for intelligent manufacturing, optoelectronic integration, and biofabrication.
- Offers high flexibility for creating advanced functional colloidal microstructures.

