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Published on: March 24, 2019
Chiral spin-liquid-like state in pyrochlore iridate thin films.
Xiaoran Liu1,2, Jong-Woo Kim3, Yao Wang4
1Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences, Beijing, China. xiaoran.liu@iphy.ac.cn.
Reduced dimensionality in pyrochlore iridates reveals a quantum disordered state in Y2Ir2O7 thin films. This state exhibits chiral spin configurations and spin-liquid-like behavior due to magnetic frustration.
Area of Science:
- Condensed Matter Physics
- Materials Science
- Quantum Materials
Background:
- Pyrochlore iridates are crucial for studying correlated and topological phenomena.
- These phenomena arise from spin-orbit coupling, electronic correlations, geometric frustration, and electron itinerancy.
- Reduced dimensionality can alter magnetic ground states, revealing exotic quantum states.
Purpose of the Study:
- To investigate the magnetic properties of Y2Ir2O7 thin films.
- To explore emergent quantum states in reduced dimensions.
- To understand the role of magnetic frustration in thin film behavior.
Main Methods:
- Magnetotransport measurements.
- Resonant elastic and inelastic x-ray scattering experiments.
- Analysis of thin film properties (thickness ≤30 nm).
Main Results:
- Discovery of an emergent quantum disordered state in Y2Ir2O7 thin films down to 5 K.
- Observation of dispersionless magnetic excitations.
- Anomalous Hall effect indicating chiral short-range spin configurations and broken time-reversal symmetry.
Conclusions:
- The chiral state originates from restored magnetic frustration in lower dimensionality.
- Competing exchange interactions and quantum fluctuations suppress long-range order.
- The findings suggest spin-liquid-like behavior with a degenerate ground-state manifold.
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