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Updated: Jun 5, 2025

Excitonic Hamiltonians for Calculating Optical Absorption Spectra and Optoelectronic Properties of Molecular Aggregates and Solids
Published on: May 27, 2020
Dynamical Exciton Condensates in Biased Electron-Hole Bilayers
Zhiyuan Sun1,2, Yuta Murakami3, Fengyuan Xuan4
1State Key Laboratory of Low-Dimensional Quantum Physics and Department of Physics, <a href="https://ror.org/03cve4549">Tsinghua University</a>, Beijing 100084, People's Republic of China.
Bilayer materials can exhibit exotic quantum phenomena. When charge tunnels between layers, exciton condensates display characteristics of the ac Josephson effect, enabling control over their light-emitting properties.
Area of Science:
- Condensed Matter Physics
- Quantum Optics
- Materials Science
Background:
- Bilayer materials can host interlayer excitons, where electrons and holes reside in separate layers.
- Maintaining a nonzero exciton density typically requires a bias chemical potential, achieved through optical pumping or electrical contacts.
Purpose of the Study:
- To investigate the behavior of exciton condensates in bilayer materials when charge tunneling is present.
- To explore the implications of the ac Josephson effect on exciton condensates.
- To examine the tunability of condensate properties and their interaction with optical cavities.
Main Methods:
- Theoretical analysis of charge tunneling in bilayer systems.
- Modeling exciton condensates within the framework of the ac Josephson effect.
- Investigating the influence of optical cavities on condensate dynamics.
Main Results:
- Demonstrated that charge tunneling leads to exciton condensates entering the dynamical regime of the ac Josephson effect.
- Identified physical consequences including measurable tunneling currents.
- Showed that condensates can be tuned from bright (photon-emitting) to dark states.
- Revealed that coupling with cavity photons can lead to superradiant phases depending on the bias.
Conclusions:
- Charge tunneling is a critical factor in the dynamical behavior of exciton condensates in bilayer materials.
- The ac Josephson effect provides a framework for understanding and controlling these condensates.
- Tunability and cavity coupling offer pathways to novel quantum optical phenomena in these systems.
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