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Updated: Jun 5, 2025

Hybrid Printing for the Fabrication of Smart Sensors
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Exploration and development of molecule-based printed electronics materials: an integrated approach using

Tatsuo Hasegawa1, Satoru Inoue1, Seiji Tsuzuki1

  • 1Department of Applied Physics, The University of Tokyo, Tokyo, Japan.

Science and Technology of Advanced Materials
|December 10, 2024
PubMed
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This summary is machine-generated.

Researchers systematically developed organic semiconductors and ferroelectrics using data and computational science, leading to novel materials with enhanced electronic properties and thin-film formability for advanced devices.

Area of Science:

  • Materials Science
  • Solid State Physics
  • Organic Electronics

Background:

  • Developing molecule-based electronic materials is hindered by unpredictable crystal structures impacting electrical properties and thin-film formation.
  • Controlling crystal structure is key to designing high-performance organic semiconductors (OSCs) and ferroelectrics.

Purpose of the Study:

  • To systematically develop crystalline organic semiconductors (OSCs) and organic ferroelectrics.
  • To integrate experimental, computational, and data sciences for material discovery and optimization.
  • To overcome challenges in crystal structure control for improved electronic and thin-film properties.

Main Methods:

  • Utilized data science for identifying promising materials from crystal structure databases.
Keywords:
Printed electronicscrystal structurecrystal structure analysisfield-effect transistororganic ferroelectricsorganic transistorquantum chemical calculationsemiconductor interface

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  • Employed computational science to clarify the origin of layered crystallinity and optimize structures.
  • Developed novel alkylated layered OSCs and molecule-based ferroelectrics.
  • Applied advanced structural analysis using cryo-electron microscopy and X-ray-free electron laser (XFEL).
  • Integrated solution processes for self-organized growth of layered OSCs.

    • Main Results:

    • Discovered unique molecule-based ferroelectrics and peculiar ferroelectric phenomena.
    • Clarified the origin of high layered crystallinity in specific molecular designs.
    • Developed OSCs with high mobility, heat resistance, and solubility.
    • Observed unique phenomena like frozen liquid crystal phases and controlled polar/antipolar order.
    • Achieved sharp, stable switching in field-effect transistors at low voltages due to clean interfaces.

    Conclusions:

    • Systematic integration of data, computational, and experimental sciences enables rational design of crystalline organic electronic materials.
    • Novel OSCs and ferroelectrics with tunable properties and enhanced performance were developed.
    • Advanced characterization techniques facilitated understanding and analysis of ultrathin crystals.
    • Developed fabrication methods yield high-performance organic electronic devices with superior interfaces.