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Non-aqueous Electrode Processing and Construction of Lithium-ion Coin Cells
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Commercially Applicable One-Step Method to Construct Homogeneous Anode/Electrolyte Interface and Cathode/Electrolyte

Jianhui Du1,2, Wanli Sha1, Chong Luo3

  • 1College of Materials Science and Engineering, Qiqihar University, Qiqihar, Heilongjiang Province 161006, China.

ACS Applied Materials & Interfaces
|December 11, 2024
PubMed
Summary

This study developed a one-step method to create dual ion-electron conductive interfaces for solid-state lithium-sulfur batteries (SLSBs), improving performance and addressing interface degradation issues for practical application.

Keywords:
dual ion-electron conductivityelectrochemical polymerizationhomogeneous Interfacein situ interfacesolid-state lithium−sulfur battery

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • Solid-state lithium-sulfur batteries (SLSBs) offer a promising solution to the shuttle effect.
  • However, SLSBs face challenges including interface degradation and poor kinetics.

Purpose of the Study:

  • To address interface degradation and kinetic issues in SLSBs.
  • To develop a novel method for simultaneously synthesizing anode/electrolyte and cathode/electrolyte interfaces.

Main Methods:

  • One-step electrochemical polymerization of thiophene monomers in poly(ethylene oxide) electrolyte.
  • In situ synthesis of dual ion-electron conductive layers on anode and cathode interfaces.

Main Results:

  • Achieved an ionic conductivity of 1.1 × 10-4 S cm-1 at 40 °C.
  • Maintained a specific capacity of 1166.6 mAh g-1 after 50 cycles.
  • Demonstrated the importance of homogeneous inner cathode surfaces and cathode/electrolyte interfaces.

Conclusions:

  • The one-step interface regulation strategy effectively enhances SLSB performance.
  • This approach offers a competitive and potentially scalable solution for SLSB technology.