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Updated: Jun 5, 2025

Characterization of Electrode Materials for Lithium Ion and Sodium Ion Batteries Using Synchrotron Radiation Techniques
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Towards High-Performance Li-Rich Cathode Materials: from Morphology Design to Electronic Structure Modulation.

Jing-Zhe Wan1, Chao Ma2, Jie-Sheng Chen1

  • 1School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai, 200240, P. R. China.

Small (Weinheim an Der Bergstrasse, Germany)
|December 16, 2024
PubMed
Summary

Lithium-rich cathode materials offer high capacity but face challenges. This review explores mechanisms and strategies, like morphology design and electronic structure modulation, to improve their performance for practical applications.

Keywords:
Li‐rich cathodesgradient structuremorphology designoxygen redoxstructure design

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • Lithium-rich cathode materials (LRMs) are promising for high-capacity batteries (exceeding 250 mAh g⁻¹).
  • Their capacity stems from transition metal (TM) ion redox and oxygen anion redox processes.
  • Key challenges include poor rate capability and voltage instability (fading and hysteresis).

Purpose of the Study:

  • To review recent mechanistic insights into lithium-rich cathode materials.
  • To discuss advancements and strategies for enhancing LRM performance.
  • To inspire future research directions for LRMs.

Main Methods:

  • Literature review of recent advancements in LRMs.
  • Analysis of strategies for performance improvement.
  • Discussion of mechanisms from morphology to electronic structure.

Main Results:

  • LRMs exhibit high reversible discharge capacity.
  • Performance limitations include rate capability and voltage issues.
  • Strategies span from material morphology to electronic structure tuning.

Conclusions:

  • Understanding LRMs' mechanisms is crucial for overcoming limitations.
  • Morphology and electronic structure modifications are key strategies.
  • Continued research is vital for realizing the practical potential of LRMs.