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Updated: Jun 5, 2025

Light-Induced In Situ Transmission Electron Microscopy for Observation of the Liquid-Soft Matter Interaction
Published on: July 26, 2022
A mixed perturbative-nonperturbative treatment for strong light-matter interactions
Carlos J Sánchez Martínez1, Johannes Feist1, Francisco J García-Vidal1,2
1Departamento de Física Teórica de la Materia Condensada and Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid, E-28049 Madrid, Spain.
Abstract:
The full information about the interaction between a quantum emitter and an arbitrary electromagnetic environment is encoded in the so-called spectral density. We present an approach for describing such interaction in any coupling regime, providing a Lindblad-like master equation for the emitter dynamics when coupled to a general nanophotonic structure. Our framework is based on the splitting of the spectral density into two terms. On the one hand, a spectral density responsible for the non-Markovian and strong-coupling-based dynamics of the quantum emitter. On the other hand, a residual spectral density including the remaining weak-coupling terms. The former is treated nonperturbatively with a collection of lossy interacting discrete modes whose parameters are determined by a fit to the original spectral density in a frequency region encompassing the quantum emitter transition frequencies. The latter is treated perturbatively under a Markovian approximation. We illustrate the power and validity of our approach through numerical simulations in three different setups, thus offering a variety of scenarios for a full test, including the ultra-strong coupling regime.
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