Nonvolatile Magnonics in Bilayer Magnetic Insulators

Nonvolatile control of spin order or spin excitations offers a promising avenue for advancing spintronics; however, practical implementation remains challenging. In this Letter, we propose a general framework to realize electrical control of magnons in 2D magnetic insulators. We demonstrate that in bilayer ferromagnetic insulators with strong spin-layer coupling, the electric field E can effectively manipulate the spin exchange interactions between the layers, enabling nonvolatile control of the corresponding magnons. Notably, in this bilayer, E can induce nonzero Berry curvature and orbital moments of magnons, the chirality of which are coupled to the direction of E. This coupling facilitates E manipulation of the corresponding magnon valley and orbital Hall currents. Furthermore, such bilayers can be easily engineered, as demonstrated by our density-functional-theory calculations on Janus bilayer Cr-based ferromagnets. Our work provides an important step toward realizing nonvolatile magnonics and paves a promising way for future magnetoelectric coupling devices.