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Updated: May 31, 2025
Synthesis and Testing of Supported Pt-Cu Solid Solution Nanoparticle Catalysts for Propane Dehydrogenation
Published on: July 18, 2017
Knowledge-driven design of boron-based catalysts for oxidative dehydrogenation of propane
Weixi Chen1, Ziyi Liu1, Lihan Zhu1
1State Key Laboratory of Fine Chemicals, Liaoning Key Laboratory for Catalytic Conversion of Carbon Resources, School of Chemistry, Dalian University of Technology, Dalian 116024, China. wangdq@dlut.edu.cn.
Abstract:
Metal-free boron-based materials exhibit remarkable performance in oxidative dehydrogenation of propane (ODHP). Rational design of boron-based catalysts requires a systematic understanding of the underlying mechanisms to constitute a knowledge base. This work provides a comprehensive view of the reaction mechanism of the boron-based ODH reaction and discusses the key features of the reaction systems, including the inhibition of deep oxidation, high olefin selectivity, and the role of water in the ODHP reaction. A perspective is provided to propose potential issues in future research, i.e. identification of hidden elementary steps for an extensive understanding of the mechanisms, and application of machine learning techniques to mine the catalyst structure-catalytic performance relationship to guide the discovery of novel boron-based materials.
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