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Ionogel Adhesives: From Structural Design to Emerging Applications.

Yangyu Huang¹, He Zhu¹, Qi Zhang¹

¹School of Science and Engineering, The Chinese University of Hong Kong, Shenzhen, Guangdong, 518172, P. R. China.

Macromolecular Rapid Communications

|February 14, 2025

Summary

Ionogel adhesives, using ionic liquids within polymer networks, offer superior bonding through non-covalent interactions. This review categorizes these advanced materials and explores future development opportunities.

Keywords:

adhesion‐enhancing strategies adhesives application ionogels

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Area of Science:

Materials Science
Polymer Chemistry
Supramolecular Chemistry

Background:

Adhesives are crucial for household and industrial applications, demanding high bonding performance.
Ionogel adhesives, combining polymer networks and ionic liquids (ILs), exhibit unique properties for enhanced adhesion.
Non-covalent interactions (ionic, ion-dipole, hydrogen bonding) within ionogels improve cohesion and substrate adhesion.

Purpose of the Study:

To provide a comprehensive review of recent advancements in ionogel adhesives.
To categorize ionogel adhesives based on their composition.
To discuss strategies for enhancing adhesive properties and highlight novel applications.

Main Methods:

Literature review and categorization of existing ionogel adhesive research.
Analysis of compositional factors influencing adhesive performance.
Identification and discussion of ionogel adhesives for specific applications.

Main Results:

Ionogels leverage ionic species to promote strong non-covalent interactions, enhancing adhesive strength.
Categorization based on composition reveals diverse strategies for tuning ionogel properties.
Novel ionogel formulations demonstrate potential for specialized, high-performance adhesive applications.

Conclusions:

Ionogel adhesives represent a significant advancement in bonding technology due to inherent non-covalent interactions.
Further research into composition-property relationships and novel applications is warranted.
The field presents numerous opportunities for developing next-generation adhesives for demanding environments.