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Low-Temperature-Sensitivity Materials for Low-Temperature Lithium-Ion Batteries.

Yuchong Ge1, Jiahe Chen1, Guozheng Ma1

  • 1School of Materials Science and Engineering, Guangdong Provincial Key Laboratory of Advanced Energy Storage Materials, South China University of Technology, Guangzhou 510640, China.

ACS Applied Materials & Interfaces
|February 19, 2025
PubMed
Summary

Tin-based materials enhance lithium-ion battery (LIB) performance in cold environments. Strategies like material regulation and electrolyte control improve low-temperature energy storage for demanding applications.

Keywords:
Sn-based materialselectrochemical kinetics reactionlithium-ion batteriessubzero temperaturetemperature sensitivity

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • Low-temperature lithium-ion batteries (LIBs) are crucial for renewable energy storage in defense and space.
  • Sn-based materials exhibit inherent low-temperature properties suitable for subfreezing energy storage.

Purpose of the Study:

  • To review principles limiting LIB performance in cold environments.
  • To present strategies for enhancing low-temperature LIB performance using Sn-based materials.

Main Methods:

  • Discussing factors like Li-ion diffusion, electrolyte viscosity, and impedance.
  • Implementing material phase transition regulation and interfacial engineering.
  • Optimizing electrolyte composition for low-temperature operation.

Main Results:

  • Identified key challenges in low-temperature LIB operation.
  • Demonstrated effectiveness of Sn-based materials and engineering strategies.
  • Proposed methods for improving cycle life and SEI formation.

Conclusions:

  • Sn-based materials offer significant potential for advanced low-temperature LIBs.
  • Material design and electrolyte engineering are key to overcoming performance limitations.
  • Future research should focus on cycle life, SEI components, and large-cell testing.