Enhanced Electrothermal Properties of Core-Sheath Lignin-Derived Carbon Nanotube Yarns with UHMWPE Insulation

A critical challenge in wearable electrothermal textiles is achieving effective insulation while maintaining sheath flexibility, which is essential for enhancing the mechanical properties and durability of conductive materials under everyday conditions, such as washing, stretching, and twisting. In this work, we employ a coaxial tubular braiding technique to coat a high-conductivity carbon nanotube (CNT) yarn with a high-strength insulation layer made of ultra-high-molecular-weight polyethylene (UHMWPE) multifilaments, resulting in a core-sheath-structure CNT yarn with excellent electrothermal performance. By adjusting the number of UHMWPE multifilaments and the sheath braiding angle, we achieve high flexibility, high tensile strength, and abrasion and wash resistance, as well as improved electrical stability for the CNT yarns. Additionally, the CNT yarns with an insulation layer effectively prevent short-circuiting during use and achieve superior thermal management, with a significant increase in steady-state temperature under operational conditions, exhibiting significant potential for applications in wearable electronic devices.