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Toward Practical All-Solid-State Batteries: Current Status of Functional Binders.

Caiwang Mao1, Jingjing Dong1, Jie Li1

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Advanced Materials (Deerfield Beach, Fla.)
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Functional binders are crucial for advancing all-solid-state batteries (ASSBs), improving electrode stability and performance. This review explores binder roles, design, and future directions for high-energy-density ASSBs.

Keywords:
all‐solid‐state batterybindercharacterizationhigh energy densitysolid electrolyte

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • All-solid-state batteries (ASSBs) offer high energy density and safety advantages over conventional lithium-ion batteries.
  • Binders are critical for electrode integrity, charge transport, and solid electrolyte interphase management in ASSBs.

Purpose of the Study:

  • To systematically review recent advancements in functional binder development for ASSBs.
  • To elucidate the roles, impacts, and failure mechanisms of binders in various ASSB components.
  • To highlight innovative binder design strategies and evaluation methodologies.

Main Methods:

  • Comprehensive literature review of binder development in ASSBs.
  • Analysis of binder functionalities in anodes, cathodes, and solid electrolytes.
  • Summary of testing methods and characterization techniques for binder performance.

Main Results:

  • Binders are essential for stabilizing electrode structures and facilitating carrier transport.
  • Functional binders are key to achieving higher energy densities in ASSBs.
  • Innovative design principles and evaluation techniques are emerging for binder optimization.

Conclusions:

  • Optimizing binder systems is a critical strategy for realizing the full potential of high-energy-density ASSBs.
  • Future research should focus on developing advanced binders tailored to specific ASSB architectures and applications.