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Field-Angle-Resolved Specific Heat in Na_{2}Co_{2}TeO_{6}: Evidence against Kitaev Quantum Spin Liquid
Shengjie Fang1, Kumpei Imamura1, Yuta Mizukami1,2
1Department of Advanced Materials Science, University of Tokyo, Kashiwa, Chiba 277-8561, Japan.
Abstract:
Kitaev quantum spin liquids (KSLs) in layered honeycomb magnets are known to host Majorana quasiparticles, whose excitations depend strongly on the direction of the applied magnetic field. In the high-field phase of α-RuCl_{3}, specific heat measurements have revealed characteristic field-angle dependence of low-energy excitations consistent with the Kitaev model, providing bulk evidence for the KSL state. Here we present low-temperature measurements of specific heat C(T) for another KSL candidate Na_{2}Co_{2}TeO_{6} (NCTO) under field rotation within the honeycomb plane. Above the critical field of antiferromagnetic order, the field-angle dependence of C/T exhibits minima along the bond directions, contrasting with the maxima observed in the KSL state of α-RuCl_{3}. Our analysis indicates nodeless, fully gapped excitations, which are inconsistent with the angle-dependent Majorana excitations with gapless nodes predicted by the Kitaev model. These findings suggest that low-energy excitations in NCTO are governed by gapped magnon excitations rather than Majorana quasiparticles, providing thermodynamic evidence against a KSL state.
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