Model-Based Prediction of the Tensile Properties of Polypropylene Films Made from Recycled Materials

This study investigates the potential of data-driven modeling to monitor and predict mechanical properties of extruded film using recyclates. The first step is to investigate whether a process parameter can indicate the input material quality of the material, which can vary significantly due to the use of recyclate. The die pressure was shown to be a key indicator due to its strong correlation with viscosity and material degradation. The second step is to explore the ability of machine learning models-Generalized Additive Models, Linear Regression, and Random Forest-to predict film tensile strength and modulus based on extrusion process and material parameters. The results demonstrate that including Melt Flow Rate and shear viscosity in addition to pressure and feedstock type (Virgin, PIR, and PCR) significantly improves model accuracy, with Generalized Additive Models achieving the highest R² of 85.7% for tensile strength prediction. Additionally, the observed variability between different recyclate streams highlights the need for a more detailed classification of recyclates to better predict and optimize the mechanical performance of the film. While data-driven approaches for predicting properties show promise, their effectiveness remains limited by data availability and feedstock variability. Expanding datasets and improving process stability will be critical to refining predictive models for industrial application.