Liquid Metal-Ionogel Core-Shell Fibers for Reflection-Suppressed Electromagnetic Interference Shielding and Strain...

Electromagnetic interference (EMI) shielding fibers are crucial in practical uses for their flexibility and one-dimensional form. However, their application is limited by poor compatibility between EMI shielding components and fiber substrates, and high electromagnetic wave reflectivity. Herein, a core/shell-structured EMI shielding fiber is introduced, featuring a core of Ga-In-Sn-Zn alloy, Carbopol, and air bubbles, and a shell of ionogel formed from copolymerized acrylamide and acrylic acid. A single fiber achieves a total shielding effectiveness of ∼35 dB within the 2-18 GHz range, which increases to ∼70 dB when three fibers are stacked. Remarkably, the fiber demonstrates enhanced EMI shielding performance following stretching and recovery. Additionally, it exhibits excellent impedance matching, with a reflection power coefficient as low as 0.14 at 10 GHz. The fiber's EMI shielding mechanism encompasses reflection shielding, absorption shielding─attributable to conduction loss and polarization loss─and multiple reflection shielding. Furthermore, the fiber shows potential as a strain sensor. This research offers an effective strategy for creating flexible fibers with high EMI shielding capabilities and low EM wave reflection.