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Metallic Solids

Metallic Solids

Metallic solids such as crystals of copper, aluminum, and iron are formed by metal atoms. The structure of metallic crystals is often described as a uniform distribution of atomic nuclei within a “sea” of delocalized electrons. The atoms within such a metallic solid are held together by a unique force known as metallic bonding that gives rise to many useful and varied bulk properties.
All metallic solids exhibit high thermal and electrical conductivity, metallic luster, and malleability....

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Updated: Jun 14, 2025

Solid-state Graft Copolymer Electrolytes for Lithium Battery Applications

Solid-state Graft Copolymer Electrolytes for Lithium Battery Applications

Published on: August 12, 2013

Lithium-Ion Conduction in Liquid-Crystalline Columnar Pd(II) Nanoassemblies.

Cristián Cuerva¹, Irene Caro-Campos¹, Mercedes Cano¹

¹Departamento de Química Inorgánica, Facultad de Ciencias Químicas, Universidad Complutense de Madrid, Ciudad Universitaria, E-28040 Madrid, Spain.

ACS Applied Materials & Interfaces

|June 12, 2025

Summary

This summary is machine-generated.

This study introduces liquid crystalline electrolytes for energy storage. Doping a palladium metallomesogen with lithium ions enhances phase stability and enables efficient Li-ion conduction.

Keywords:

Li-ion conduction columnar mesophase liquid crystals metallomesogens nanoassemblies

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Synthesis of Ionic Liquid Based Electrolytes, Assembly of Li-ion Batteries, and Measurements of Performance at High Temperature

Synthesis of Ionic Liquid Based Electrolytes, Assembly of Li-ion Batteries, and Measurements of Performance at High Temperature

Published on: December 20, 2016

Area of Science:

Materials Science
Electrochemistry
Supramolecular Chemistry

Background:

Liquid crystalline electrolytes offer anhydrous operation and high-temperature stability for energy storage.
Metallomesogens, specifically bispyrazolate Pd(II) compounds, can form ordered mesophases suitable for ion conduction.

Purpose of the Study:

To investigate the use of a bispyrazolate Pd(II) metallomesogen as a platform for lithium-ion (Li-ion) conduction.
To explore the effect of lithium doping on the mesomorphic properties and ionic conductivity of the metallomesogen.

Main Methods:

Preparation of Li-doped liquid crystal composites with varying lithium content.
Characterization of mesomorphic properties (melting and clearing points).
Measurement of ionic conductivity using complex impedance spectroscopy.

Main Results:

Lithium ion intercalation stabilized the hexagonal columnar mesophase, extending its temperature range.
Ion-dipole interactions between Li+ ions and the metallomesogen enhanced phase stability.
High Li-ion conductivity (up to 1.89 × 10^-4 Ω^-1 cm^-1) was achieved in both solid and liquid crystalline states.

Conclusions:

Bispyrazolate Pd(II) metallomesogens are promising candidates for developing novel liquid crystalline Li-ion electrolytes.
The ordered nanochannels within the mesophase facilitate efficient Li-ion transport.
This research opens avenues for advanced anhydrous electrolytes in energy storage devices.