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Updated: Sep 18, 2025

Excitonic Hamiltonians for Calculating Optical Absorption Spectra and Optoelectronic Properties of Molecular Aggregates and Solids
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Extracting Coupling-Mode Spectral Densities with Two-Dimensional Electronic Spectroscopy

Roosmarijn de Wit1, Jonathan Keeling1, Brendon W Lovett1

  • 1SUPA, School of Physics and Astronomy, University of St Andrews, St Andrews KY16 9SS, United Kingdom.

The Journal of Physical Chemistry Letters
|June 20, 2025
PubMed
Summary

This study introduces a new method using two-dimensional electronic spectroscopy to extract the full vibrational spectral density, revealing environmental impacts on molecular function. The technique highlights the crucial role of non-Markovian dynamics in understanding these interactions.

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