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We demonstrate spin-polarized helical edge transport in graphene at zero magnetic field using CrPS4. This breakthrough enables robust quantum spin Hall states and magnetism, paving the way for spintronic devices.

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Area of Science:

  • Condensed Matter Physics
  • Materials Science
  • Spintronics

Background:

  • Long-distance coherent spin propagation is crucial for spintronics.
  • Topological spin-polarized edge states in graphene offer a promising route.
  • Engineering graphene's band structure via van der Waals heterostructures is key for achieving these states without external magnetic fields.

Purpose of the Study:

  • To detect spin-polarized helical edge transport in graphene at zero external magnetic field.
  • To investigate the coexistence of quantum spin Hall (QSH) states and magnetism in graphene.
  • To explore the potential for practical applications in quantum spintronic circuitries.

Main Methods:

  • Utilizing van der Waals heterostructures with an interlayer antiferromagnet, CrPS4, to induce proximity effects in graphene.
  • Engineering graphene's band structure to create a topological bulk gap with gapless helical edge states.
  • Experimental detection of spin-polarized helical edge transport and anomalous Hall (AH) effect.

Main Results:

  • Successful detection of spin-polarized helical edge transport in graphene at zero external magnetic field.
  • Demonstration of the coexistence of quantum spin Hall (QSH) states and magnetism in graphene.
  • Observation of a large anomalous Hall (AH) effect due to induced spin-orbit and exchange couplings, persisting up to room temperature.

Conclusions:

  • The proximity of CrPS4 enables the formation of QSH states in graphene without external magnetic fields.
  • The observed QSH states and room-temperature AH effect in magnetic graphene open avenues for spintronic applications.
  • This work provides a pathway for developing practical quantum spintronic circuitries based on engineered magnetic graphene.