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    Thulium-doped YLF crystals were optimized for 1.5 µm laser operation. A cascade laser scheme successfully suppressed self-termination, enabling efficient continuous-wave laser output.

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    Area of Science:

    • Materials Science
    • Laser Physics
    • Spectroscopy

    Background:

    • Continuous-wave (CW) laser operation around 1.5 µm is crucial for various applications, including telecommunications and medical treatments.
    • Thulium (Tm³⁺)-doped materials are promising candidates for generating laser light in this wavelength range.
    • Self-termination due to long-lived lower laser levels can hinder efficient CW laser performance.

    Purpose of the Study:

    • To investigate Tm³⁺-doped YLF crystals for CW laser operation at 1.5 µm.
    • To analyze spectroscopic properties and optimize doping concentrations.
    • To circumvent laser self-termination using a cascade laser scheme.

    Main Methods:

    • Growth of Tm³⁺-doped YLF crystals with varying doping concentrations.
    • Spectroscopic investigations including emission, absorption, and gain cross-section measurements.
    • Characterization of concentration-dependent lifetime of energy levels.
    • Implementation of a cascade laser scheme (³H₄→³F₄→³H₆) to depopulate the lower laser level.
    • Ti:sapphire laser pumping at 781 nm.

    Main Results:

    • Spectroscopic data (emission, absorption, gain cross sections, lifetimes) were obtained.
    • The cascade laser scheme effectively depopulated the lower laser level (³F₄).
    • Simultaneous CW laser operation was achieved at 1509 nm and 1923 nm.
    • Slope efficiencies of 44% (1509 nm) and 35% (1923 nm) were recorded.
    • Maximum output powers reached 590 mW (1509 nm) and 670 mW (1923 nm).

    Conclusions:

    • Tm³⁺-doped YLF crystals are suitable for efficient CW laser operation around 1.5 µm.
    • The cascade laser scheme is an effective strategy to overcome self-termination in Tm³⁺ lasers.
    • Optimized Tm³⁺-doped YLF crystals offer promising performance for 1.5 µm laser applications.