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Isomers are different chemical species that have the same chemical formula. Structural isomerism of coordination compounds can be divided into two subcategories, the linkage isomers and coordination-sphere isomers.
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Organometallic compounds are compounds that contain a carbon–metal bond. Carbon belongs to an organyl group like alkyl, aryl, allyl, or benzyl groups. The metal can be from Group I or Group II of the periodic table, a transition metal, or a semimetal.
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Isoreticular moiré metal-organic frameworks with quasiperiodicity.

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Researchers created quasiperiodic patterns in metal-organic frameworks (MOFs) by twisting layers. Ligand design allowed control over pattern length scales, offering new possibilities for functional moiré materials.

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Area of Science:

  • Materials Science
  • Crystallography
  • Chemistry

Background:

  • Quasicrystals exhibit unique, non-repeating atomic structures with forbidden rotational symmetries.
  • Controlling quasiperiodic length scales in materials is challenging due to atomic and chemical constraints.

Purpose of the Study:

  • To utilize metal-organic frameworks (MOFs) as a platform for generating quasiperiodic moiré patterns.
  • To demonstrate systematic control over the characteristic length scales of these patterns through rational design.

Main Methods:

  • Employing twisted bilayer structures within MOFs to create moiré patterns.
  • Utilizing rational ligand design based on isoreticular principles for structural modulation.
  • Characterizing patterns using high-resolution transmission electron microscopy (HR-TEM) and mathematical analysis.

Main Results:

  • Successfully generated moiré patterns with dodecagonal quasiperiodic symmetry in MOFs.
  • Demonstrated systematic modulation of pattern length scales via ligand modification.
  • Observed patterns resemble quasicrystals but arise from layer stacking, not intrinsic order.

Conclusions:

  • Reticular chemistry can incorporate quasiperiodicity into material design.
  • This approach expands the structural design space for functional moiré materials.
  • The study provides a conceptual framework for creating complex ordered structures.