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Related Concept Videos

Olefin Metathesis Polymerization: Acyclic Diene Metathesis (ADMET)00:53

Olefin Metathesis Polymerization: Acyclic Diene Metathesis (ADMET)

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Acyclic diene metathesis polymerization or ADMET polymerization involves cross-metathesis of terminal dienes, such as 1,8-nonadiene, to give linear unsaturated polymer and ethylene. As ADMET is a reversible process, the formed ethylene gas must be removed from the reaction mixture to complete the polymerization process.
Similar to cross-metathesis, ADMET also involves the formation of metallacyclobutane intermediate by [2+2] cycloaddition of one of the double bonds of a terminal diene with...
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Related Experiment Video

Updated: Sep 10, 2025

Designed for Molecular Recycling: A Lignin-Derived Semi-aromatic Biobased Polymer
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Designed for Molecular Recycling: A Lignin-Derived Semi-aromatic Biobased Polymer

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Reversible biobased adhesives enable closed-loop engineered composites.

Jin Lv1, Daxin Zhang2, Xinkai Li1

  • 1National Key Laboratory of Advanced Polymer Materials, Polymer Research Institute, Sichuan University, Chengdu, China.

Nature Communications
|August 23, 2025
PubMed
Summary
This summary is machine-generated.

Researchers developed a novel biobased adhesive using cellulose nanoconfinement. This ultra-strong, recyclable adhesive offers switchable adhesion, reducing environmental impact and enabling closed-loop systems for engineered composites.

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Area of Science:

  • Materials Science
  • Green Chemistry
  • Polymer Science

Background:

  • Petrochemical-based synthetic resin adhesives pose environmental and health risks.
  • Developing sustainable, biomass-derived adhesives with strong adhesion is a key research area.
  • Recycling challenges exist for current strong adhesives, particularly hetero-layered composites.

Purpose of the Study:

  • To create an ultra-strong yet switchable biobased adhesive using a supramolecularly connected nanoconfined network.
  • To enable efficient recycling of adhesive-based composites through a dynamic crosslinked network.
  • To assess the environmental and health benefits of the proposed adhesive strategy.

Main Methods:

  • Utilized cellulose nanoconfinement (36.5-46.3 wt%) within a supramolecular network.
  • Incorporated thermally responsive disulfide bonds for switchable adhesion.
  • Evaluated adhesion strength, thermo-responsive detachment, and recyclability.

Main Results:

  • Achieved excellent adhesion strength (6.02 MPa), supporting 65 kg on 4 cm².
  • Demonstrated instant thermo-responsive detachment (switching ratio > 600, response time ≤ 10 s).
  • Enabled full disassembly and recycling of composites via dynamic network destruction.

Conclusions:

  • The nanoconfined network strategy provides ultra-strong, switchable, and recyclable biobased adhesives.
  • This approach significantly reduces environmental (7.52 * 10² PAF m³ d/kg emitted) and health (2.04 * 10⁻⁴ cases/kg emitted) burdens.
  • Establishes a paradigm for closed-loop engineered composites, offering a breakthrough in green intelligent adhesives.