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Preparation and Reactions of Sulfides02:26

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Sulfides are the sulfur analog of ethers, just as thiols are the sulfur analog of alcohol. Like ethers, sulfides also consist of two hydrocarbon groups bonded to the central sulfur atom. Depending upon the type of groups present, sulfides can be symmetrical or asymmetrical. Symmetrical sulfides can be prepared via an SN2 reaction between 2 equivalents of an alkyl halide and one equivalent of sodium sulfide.
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A type of Lewis acid-base chemistry involves the formation of a complex ion (or a coordination complex) comprising a central atom, typically a transition metal cation, surrounded by ions or molecules called ligands. These ligands can be neutral molecules like H2O or NH3, or ions such as CN− or OH−. Often, the ligands act as Lewis bases, donating a pair of electrons to the central atom. These types of Lewis acid-base reactions are examples of a broad subdiscipline called coordination...
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A battery is a galvanic cell that is used as a source of electrical power for specific applications. Modern batteries exist in a multitude of forms to accommodate various applications, from tiny button batteries such as those that power wristwatches to the very large batteries used to supply backup energy to municipal power grids. Some batteries are designed for single-use applications and cannot be recharged (primary cells), while others are based on conveniently reversible cell reactions that...
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On comparing the reactivity of silver and lead, it is observed that the two ionic species, Ag+ (aq) and Pb2+ (aq), show a difference in their redox reactivity towards copper: the silver ion undergoes spontaneous reduction, while the lead ion does not. This relative redox activity can be easily quantified in electrochemical cells by a property called cell potential. This property is commonly known as cell voltage in electrochemistry, and it is a measure of the energy which accompanies the charge...
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Solid-state Graft Copolymer Electrolytes for Lithium Battery Applications
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High Performance Sulfide Solid-State Battery Electrolytes Regulation Mechanism: A Review.

Keyu Chen1, Yuchuan Zhu1, Jiayang Li1

  • 1College of Chemistry and Materials Engineering, Wenzhou University, Wenzhou, 325035, China.

Angewandte Chemie (International Ed. in English)
|September 9, 2025
PubMed
Summary
This summary is machine-generated.

Sulfide solid electrolytes (SEs) offer high conductivity for all-solid-state batteries (ASSBs). This review details strategies to enhance SE stability and performance, addressing key challenges for future development.

Keywords:
All‐solid‐state batteriesChemical stabilityGlass structure theorySoft–hard‐acid–base theorySulfide solid electrolyte

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Solid-state Chemistry

Background:

  • Sulfide solid electrolytes (SEs) possess high ionic conductivity and mechanical strength.
  • Poor air stability and solid-solid contact hinder the application of sulfide all-solid-state batteries (ASSBs).

Purpose of the Study:

  • To review the historical development and major breakthroughs of sulfide SEs.
  • To discuss theories and strategies for improving the chemical stability of sulfide SEs.
  • To explore thermal runaway and reaction mechanisms for enhanced stability and conductivity.

Main Methods:

  • Literature review of sulfide SE development.
  • Discussion of hard-soft-acid-base and glass structure theories.
  • Analysis of thermodynamic and kinetic aspects of SE mechanisms.

Main Results:

  • Identified key strategies for improving sulfide SE chemical stability.
  • Provided insights into thermal runaway and reaction mechanisms.
  • Highlighted current challenges and future research directions.

Conclusions:

  • Sulfide SEs are promising for ASSBs but require stability improvements.
  • Further research on stability, conductivity, and interface engineering is crucial.
  • This review offers a reference for advancing sulfide SE technology.