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Updated: Jan 18, 2026

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2D Active Filler Modified Porous Polymer Network for Stabilizing Zn Anode Under Harsh Conditions.

Haifeng Bian1, Changhao Wang2,3, Shunshun Jia1

  • 1National Laboratory of Solid State Microstructures, Collaborative Innovation Center of Advanced Microstructures, Jiangsu Key Laboratory of Artificial Functional Materials, College of Engineering and Applied Sciences, Nanjing University, Nanjing, 210093, P. R. China.

Small (Weinheim an Der Bergstrasse, Germany)
|September 10, 2025
PubMed
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This summary is machine-generated.

This study introduces zirconium phosphate (ZrP) as a 2D filler to improve zinc anode performance in batteries. The enhanced porous polymer coating significantly boosts ion transport, enabling longer cycle life under demanding conditions.

Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • Artificial porous polymer coatings show potential for Zn anodes but suffer from low ion transport.
  • This limitation hinders performance under harsh conditions like high current density and depth of discharge (DOD).

Purpose of the Study:

  • To enhance Zn2+ migration and protective effects in porous polymer coatings for Zn anodes.
  • To improve the stability and cycle life of Zn anodes under challenging operating conditions.

Main Methods:

  • Incorporation of a 2D active filler, zirconium phosphate (ZrP), into a porous poly(methylmethacrylate) (PPMMA) network.
  • Characterization of the modified coating's ion transport properties and protective capabilities.

Main Results:

Keywords:
2D ion conductorZn anodeZn2+ migrationcomposite coatingporous polymer networkside reaction

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  • ZrP accelerates Zn2+ transport within the PPMMA network due to its interlayer channels and zincophilicity.
  • The modified PPMMA/ZrP coating significantly enhances Zn anode reversibility and protective effects.
  • Achieved ultra-long cycle lifespan: 1000 h at 10 mA cm-2 (DOD = 5.7%) and 280 h at 20 mA cm-2 (DOD = 56.9%).
  • Full cells with PPMMA/ZrP coated ultra-thin Zn anodes (10 µm) demonstrated over 3000 cycles of stable performance.

Conclusions:

  • The 2D ZrP filler effectively optimizes Zn2+ migration in porous polymer coatings.
  • The PPMMA/ZrP composite coating provides a promising strategy for developing high-performance and stable Zn anodes for energy storage applications.