Multimode Input Enhancement of Absorption Sensing of Methane in a Hollow Bottle Microresonator

Dissipative sensing in a whispering-gallery-mode (WGM) microresonator entails monitoring changes in WGM throughput dip depth or linewidth due to analyte absorption. In our earlier work, we showed that dip depth sensitivity can be two orders of magnitude greater than linewidth sensitivity for sensing the broadband absorption of a dye in methanol. Here we experimentally demonstrate enhancement of absorption sensing of methane. Its narrowband absorption lines (a few GHz linewidth) necessitate strain tuning of the WGM of our hollow bottle resonator (HBR) to bring the WGM into resonance with the absorption line. Three asymmetric tapered fibers with different nonadiabaticities were designed to excite multiple fiber modes that couple into the WGM to interact with methane inside the HBR via the internal evanescent field. Measurements were carried out for both pure and trace (in 1 atm of air) methane at 1654 and 1651 nm. Enhancement factors as large as 141 were found; the experimental results agree with theoretical calculations and with the predictions of a limiting-case model. Effective absorption path lengths as large as 273 cm, more than ten thousand times the HBR diameter, were achieved for trace methane sensing, with detection limits estimated to be in the hundreds of ppm.