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High-Performance Dendrite-Free Lithium Textile Anodes Using Interfacial Interaction-Mediated Ultrathin Metal Organic

Donghyeon Nam1,2, Gwonho Yu3, Chanseok Lee1

  • 1Department of Chemical and Biological Engineering, Korea University, 145 Anam-ro, Seongbuk-gu, Seoul, 02841, Republic of Korea.

Advanced Materials (Deerfield Beach, Fla.)
|September 13, 2025
PubMed
Summary
This summary is machine-generated.

Researchers developed a dendrite-free lithium metal anode using ultrathin metal-organic framework multilayers. This innovation enhances battery stability and capacity for next-generation energy storage.

Keywords:
Li textile anodeMOF multilayerscoordination‐bonding layer‐by‐layer assembly

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Nanotechnology

Background:

  • Lithium metal batteries offer high energy density but face safety challenges due to lithium dendrite growth.
  • Developing stable and high-capacity lithium metal anodes is crucial for next-generation batteries.

Purpose of the Study:

  • To introduce a high-performance, dendrite-free lithium metal textile anode.
  • To enhance the stability and capacity of lithium metal batteries through interfacial engineering.

Main Methods:

  • Fabrication of ultrathin metal-organic framework (MOF) multilayers on polyester textiles via layer-by-layer assembly of silver ions and trithiocyanuric acid.
  • In situ reduction of silver ions to silver nanoparticles for improved lithium nucleation.
  • Formation of a Li3N-rich solid electrolyte interphase layer.

Main Results:

  • Achieved a uniform, ultrathin MOF multilayer (<40 nm) on a textile anode.
  • Demonstrated in situ formation of highly lithiophilic silver nanoparticles, lowering the lithium nucleation energy barrier.
  • Exhibited exceptional stability over 2000 hours in a symmetric cell and ≈96.5% capacity retention after 1300 cycles in a full cell.

Conclusions:

  • The developed MOF multilayer approach effectively suppresses lithium dendrite growth.
  • Interfacial interactions and ultrathin lithiophilic layers are critical for advancing lithium metal battery performance.
  • This strategy offers a promising pathway for developing safer and more stable high-energy-density batteries.