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Bayesian inference of anisotropic 2D small-angle scattering from sparse measurement
Chi-Huan Tung1, Yangyang Wang2, Jan-Michael Carrillo2
1Neutron Scattering Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA.
The Journal of Chemical Physics
|October 15, 2025
Summary
We developed a new Bayesian method to reconstruct 2D small-angle scattering (SAS) patterns from limited data. This technique accurately recovers structural details, even with sparse or noisy measurements, improving material analysis.
Area of Science:
- Materials Science
- Neutron Scattering Physics
- Computational Physics
Background:
- Two-dimensional small-angle scattering (2D SAS) is crucial for analyzing material structures.
- Current methods struggle with sparse, noisy, or incomplete 2D SAS data.
- Reconstructing accurate patterns is essential for quantitative structural analysis.
Purpose of the Study:
- To present a novel Bayesian inference framework for reconstructing 2D SAS patterns.
- To enable accurate pattern reconstruction from limited, noisy, or partially missing data.
- To enhance the applicability of 2D SAS techniques under challenging experimental conditions.
Main Methods:
- A Bayesian inference framework combining a symmetry-aware angular basis.
- Radial Gaussian process priors for training-free interpolation and denoising.
- Computational benchmarks and experimental validations on various materials.
Main Results:
- Reliable recovery of isotropic and anisotropic features from severely reduced data.
- Improved fidelity and resolution compared to raw 2D SAS measurements.
- Achieved comparable accuracy with up to 50-fold fewer detected neutrons.
Conclusions:
- The framework enables quantitative structural analysis under low-flux, time-limited, or single-shot conditions.
- Extends 2D SAS applicability to compact neutron sources.
- Facilitates the study of soft matter systems with transient structural changes.
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