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Solid-State Lithium Metal Batteries with Improved Performance via Polymer Electrolyte Interface Modification.

Preeti Yadav1, Pallavi Thakur1, Lily Mandal2

  • 1Tata Institute of Fundamental Research Hyderabad, Sy No 36/P Serilingampally Mandal, Hyderabad 500046, India.

ACS Applied Materials & Interfaces
|October 23, 2025
PubMed
Summary
This summary is machine-generated.

Researchers developed a stable solid electrolyte interface for lithium metal batteries by modifying the lithium metal surface. This enables ambient assembly, enhancing battery safety and reducing costs for high-performance applications.

Keywords:
Air StabilityArtificial SEILithium FluorideLithium Metal BatteriesSolid Polymer Electrolyte

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Battery Technology

Background:

  • Lithium metal batteries (LMBs) offer high energy density but face challenges with safety and ambient assembly.
  • Developing a stable solid electrolyte interface (SEI) is crucial for overcoming these limitations.

Purpose of the Study:

  • To demonstrate a method for modifying lithium metal surfaces to create a stable SEI.
  • To enable ambient assembly of LMBs, improving safety and reducing manufacturing costs.

Main Methods:

  • Surface modification of lithium metal (LM) using direct and polymer electrolyte approaches.
  • Hot pressing in air to form a stable SEI with *in situ* LiF and defective graphene.
  • Utilizing an optimized thin film of fluorinated graphite polymer.

Main Results:

  • Achieved enhanced cyclability (>1000 cycles for Li||Li, >200 cycles for Li||NMC) at high current densities.
  • Demonstrated a high Li+ transference number (0.62 ± 0.08) at room temperature.
  • Improved air stability and fire resistance of the lithium anode.

Conclusions:

  • The developed SEI modification enables air-stable lithium anodes and facilitates ambient assembly of LMBs.
  • This approach significantly enhances battery cyclability and safety, addressing key concerns with metallic lithium.
  • The method paves the way for low-cost, high-performance lithium metal batteries.