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Quantum interference and occupation control in high harmonic generation from monolayer WS2.

Minjeong Kim1,2, Taeho Kim1,2, Anna Galler3,4

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Researchers explored quantum interference in two-dimensional hexagonal materials like WS2. Intense laser fields revealed how electrons across the entire Brillouin zone influence high harmonic generation, advancing quantum technologies.

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Area of Science:

  • Condensed Matter Physics
  • Quantum Optics
  • Materials Science

Background:

  • Two-dimensional hexagonal materials possess valley degrees of freedom crucial for quantum computing and optoelectronics.
  • Nonlinear optics utilizes K and K' valleys for ultrafast control of excitons and quantum phenomena.
  • The behavior of coherent carrier dynamics away from K/K' valleys under intense laser fields remains largely uninvestigated.

Purpose of the Study:

  • To investigate quantum interferences in high harmonic generation (HHG) from monolayer WS2.
  • To explore the role of coherent carrier dynamics across the full Brillouin zone under strong laser fields.
  • To understand how electrons beyond the K/K' valleys contribute to HHG.

Main Methods:

  • Experimental observation of high harmonic generation in monolayer WS2.
  • Application of intense laser fields to drive electrons across the Brillouin zone.
  • Comparison of experimental results with quantum simulations.

Main Results:

  • Quantum interferences were observed in HHG from monolayer WS2.
  • In the perturbative regime, valley resonances enhanced HHG via multi-photon excitations.
  • In the strong-field regime, HHG was controlled by quantum interferences involving electrons across the full Brillouin zone, including regions far from the K/K' valleys.

Conclusions:

  • Experimental findings align strongly with quantum simulations, validating the interpretation.
  • This study reveals new methods for utilizing laser-driven quantum interference in 2D hexagonal systems.
  • Proposes all-optical techniques to probe and control electronic structures throughout the Brillouin zone using strong-field nonlinear optics, benefiting quantum technologies.