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Recyclable Turing-Structured Polymer Electrolytes for Sustainable Solid-State Batteries.

Jingteng Zhao1, Zhongqiang Wang1, Cong Tian1

  • 1Shandong Provincial Key Laboratory for Science of Material Creation and Energy Conversion, Science Center for Material Creation and Energy Conversion, Institute of Frontier Chemistry, School of Chemistry and Chemical Engineering, Shandong University, Qingdao, P.R. China.

Angewandte Chemie (International Ed. in English)
|November 18, 2025
PubMed
Summary
This summary is machine-generated.

This study introduces a recyclable Turing-structured polymer electrolyte (TPE) that overcomes limitations in solid polymer electrolytes. TPEs offer high ionic conductivity and stable low-temperature performance, with excellent recyclability for sustainable batteries.

Keywords:
Ionic conductivityRecyclabilitySolid polymer electrolytesSolid‐state batteriesTuring structures

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Polymer Chemistry

Background:

  • Solid polymer electrolytes (SPEs) exhibit limitations in ionic conductivity, ion transference, and recyclability.
  • Developing advanced electrolytes is crucial for high-performance solid-state batteries.

Purpose of the Study:

  • To engineer a recyclable Turing-structured polymer electrolyte (TPE) with enhanced ionic conductivity and stability.
  • To address the limitations of conventional SPEs for sustainable energy storage.

Main Methods:

  • Fabrication of TPEs via gas/liquid/solid interface using evaporation/diffusion-driven instability.
  • Characterization of the Turing structure for ion conduction pathways and Li+ self-concentration.
  • Evaluation of electrochemical performance in solid-state batteries at various temperatures and recyclability.

Main Results:

  • Achieved high Li+ conductivity (1.6 × 10-3 S cm-1 at 25°C) and transference number (0.61) due to the 3D percolating Li+ conduction facilitated by the Turing structure.
  • Demonstrated stable cycling performance in solid-state batteries at -20°C.
  • Showcased excellent self-healing, flame-retardant, and recyclable properties, with 86.5% polymer precursor and 82.6% LiTFSI salt recovery.

Conclusions:

  • Turing-structured polymer electrolytes offer a scalable design for sustainable and high-performance energy storage.
  • The developed TPEs overcome critical limitations of SPEs, enabling efficient and recyclable solid-state batteries.
  • This work highlights the potential of interface-driven self-assembly for advanced functional materials.