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A type of Lewis acid-base chemistry involves the formation of a complex ion (or a coordination complex) comprising a central atom, typically a transition metal cation, surrounded by ions or molecules called ligands. These ligands can be neutral molecules like H2O or NH3, or ions such as CN− or OH−. Often, the ligands act as Lewis bases, donating a pair of electrons to the central atom. These types of Lewis acid-base reactions are examples of a broad subdiscipline called coordination...
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Binder-Free, Self-Supporting, and Highly Conductive Sulfide Electrolytes Enabling Superior Anode Stability.

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Summary

Researchers developed a binder-free sulfide-based glass solid electrolyte (SE) using warm isostatic pressing (WIP). This advancement enables high-performance all-solid-state batteries (ASSBs) with enhanced safety and energy density.

Keywords:
all‐solid‐state batteriesbinder‐lessglass ceramicsself‐supporting membranesulfide‐based solid electrolytes

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • All-solid-state batteries (ASSBs) promise higher energy density, power, and safety than conventional lithium-ion batteries.
  • Developing solid electrolytes (SEs) with high ionic conductivity and stability is crucial for ASSB realization.

Purpose of the Study:

  • To fabricate a robust sulfide-based glass SE layer using warm isostatic pressing (WIP).
  • To integrate the SE into practical ASSB devices and evaluate their performance.

Main Methods:

  • Fabrication of a binder-free sulfide-based glass SE layer via warm isostatic pressing (WIP).
  • Incorporation of a glass-based supporting layer for mechanical enhancement.
  • Integration of SE layers into 13 mAh-class laminated ASSBs with Ni-Co-Mn cathodes and graphite anodes.

Main Results:

  • WIP process efficiency was enhanced by eliminating binders.
  • The glass-based supporting layer provided mechanical strength and flexibility to the SE film.
  • Assembled ASSBs retained ~80% capacity after 300 cycles at 25°C and 20 MPa stack pressure.

Conclusions:

  • Binder-free SE fabrication using WIP is a viable strategy for ASSBs.
  • The developed SE layers facilitate the creation of high-performance, stable ASSBs.
  • This work paves the way for practical, high-performance ASSB implementation.