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Potential-Driven Selective Na Metal Deposition-Enabled Interphase with High Lithium Dendrite Suppression Capability.

Hongli Wan^1,2, Chi Chen³, Ni Zhang^1,2

¹Ningbo Institute of Materials Technology & Engineering, Chinese Academy of Sciences, 315201 Ningbo, China.

Journal of the American Chemical Society

|November 21, 2025

Summary

This summary is machine-generated.

This study introduces a novel interlayer and anode strategy for all-solid-state Li-metal batteries (ASSLBs). This approach simultaneously tackles void formation and lithium dendrite growth, enhancing battery stability under low pressure.

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Area of Science:

Materials Science
Electrochemistry
Energy Storage

Background:

All-solid-state Li-metal batteries (ASSLBs) face challenges with void formation during Li stripping and Li dendrite growth during plating.
These issues limit ASSLB stability, especially under low stack pressure, hindering practical application.

Purpose of the Study:

To simultaneously address void formation and Li dendrite growth in ASSLBs.
To develop a stable cycling performance for ASSLBs under low stack pressure.

Main Methods:

Utilized a hard carbon-Sn (HC-Sn) interlayer and LiNa as the anode.
Investigated the in situ structural transformation to Li₆PS₅Cl/[HC-Li_xSn]Na/Na/LiNa.
Evaluated symmetric cell performance and full cell cycling stability.

Main Results:

Achieved uniform Li deposition and suppressed void formation through the HC-Sn interlayer and LiNa anode.
Demonstrated stable Li plating/stripping for 1184 hours in a symmetric cell under low stack pressure (2.0 MPa).
A full cell exhibited 90.0% capacity retention after 1000 cycles and high reversible capacity.

Conclusions:

The HC-Sn interlayer and LiNa anode strategy effectively suppresses Li dendrites and void formation.
This approach enables stable ASSLB cycling performance under low stack pressure, paving the way for practical applications.