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Area of Science:

  • Electrochemistry
  • Electrocatalysis
  • Green Chemistry

Background:

  • Electrochemistry is vital for energy storage and chemical production using renewable energy.
  • Understanding electrode-electrolyte interfaces is key for designing efficient electrocatalytic systems.
  • Recent advancements address stability challenges in electrocatalysis.

Purpose of the Study:

  • To provide a comprehensive overview of electrode processes in electrochemistry.
  • To link the historical development of electrochemistry with its future applications.
  • To offer fundamental insights for designing efficient electrochemical reactions.

Main Methods:

  • Discussion of microkinetic modeling with and without rate-determining step assumptions.
  • Analysis of mass transport effects and electrode material reconstruction.
  • Exploration of microkinetic models for degradation processes and graph theory for reaction mechanisms.
  • Introduction of data-driven approaches for activity and stability analysis.
  • Proposal of a heuristic framework for organizing electrode states.

Main Results:

  • Provides a structured understanding of electrode processes, from basic principles to advanced modeling.
  • Integrates historical context with modern data-driven techniques for electrocatalysis.
  • Offers a framework for analyzing electrode states and degradation phenomena.

Conclusions:

  • The review offers fundamental insights into electrified electrode-electrolyte interfaces.
  • It aims to inspire the rational design of highly efficient electrochemical reactions for green chemistry.
  • This work serves as a valuable resource for students and researchers in electrochemistry.