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Area of Science:

  • Materials Science
  • Electrochemistry
  • Energy Storage

Background:

  • Solid-state lithium metal batteries (SSLMBs) offer high energy density and safety.
  • Sluggish charge transfer kinetics in heterogeneous solid components limit practical performance.
  • Improving charge transport is crucial for advancing SSLMB technology.

Purpose of the Study:

  • To review and propose multi-level structural modulation strategies for optimizing charge transport in SSLMBs.
  • To analyze factors impacting structural regulation and principles for charge transport enhancement.
  • To provide insights into developing high-performance inorganic SSLMBs.

Main Methods:

  • Literature review and evaluation of multi-level structural modulation techniques.
  • Analysis of structure-charge transport-performance relationships.
  • Comparative assessment of different structural modulation approaches for charge transport.

Main Results:

  • Summarized research progress in multi-level structural modulation for SSLMBs.
  • Identified key factors and principles for structural regulation at electrode, electrolyte, and cell levels.
  • Evaluated the enhancement and limitations of various structural modulation methods.

Conclusions:

  • Multi-level structural modulation is essential for optimizing charge transport in SSLMBs.
  • Understanding and applying regulation principles can significantly improve electrochemical performance.
  • This review offers guidelines for developing next-generation high-performance inorganic SSLMBs.