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Sub-tesla On-Chip Nanomagnetic Metamaterial Platform for Angle-Resolved Photoemission Spectroscopy.

Wenxin Li1, Wisha Wanichwecharungruang2, Mingyang Guo3

  • 1Department of Applied Physics, Yale University, New Haven, Connecticut 06511, United States.

The Journal of Physical Chemistry Letters
|December 11, 2025
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Summary
This summary is machine-generated.

Researchers developed a new method using nanomagnetic metamaterial substrates to apply magnetic fields during angle-resolved photoemission spectroscopy (ARPES) measurements. This technique minimizes photoelectron trajectory distortion, enabling detailed study of magnetic field effects on quantum materials.

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Area of Science:

  • Condensed Matter Physics
  • Materials Science
  • Quantum Materials

Background:

  • Magnetically controlled states in quantum materials dictate their electronic and magnetic properties.
  • Angle-resolved photoemission spectroscopy (ARPES) is crucial for visualizing these states but is disrupted by magnetic fields affecting photoelectron trajectories.

Purpose of the Study:

  • To develop an *in situ* method for applying magnetic fields during ARPES measurements.
  • To overcome the limitations of photoelectron trajectory distortion caused by external magnetic fields.

Main Methods:

  • Utilized substrates made of nanomagnetic metamaterial arrays with alternating polarity.
  • Generated strong, homogeneous, and spatially confined magnetic fields (up to 1 T) for sample analysis.
  • Applied the method to samples up to micron thickness, including monolayer graphene.

Main Results:

  • Successfully enabled ARPES measurements under applied magnetic fields.
  • Demonstrated minimal photoelectron trajectory distortion, validated with ARPES data on monolayer graphene.
  • Achieved state-of-the-art energy-momentum resolution for magnetic field-dependent studies.

Conclusions:

  • The novel substrate method allows for direct visualization of magnetic field-controlled electronic structures.
  • This technique facilitates the study of field-tunable quantum phases in quantum materials.
  • Opens new avenues for high-resolution ARPES investigations under magnetic fields.